Robust evidence for reversal of the trend in aerosol effective climate forcing

Author:

Quaas JohannesORCID,Jia HailingORCID,Smith ChrisORCID,Albright Anna LeaORCID,Aas WencheORCID,Bellouin NicolasORCID,Boucher OlivierORCID,Doutriaux-Boucher Marie,Forster Piers M.,Grosvenor DanielORCID,Jenkins StuartORCID,Klimont Zbigniew,Loeb Norman G.,Ma XiaoyanORCID,Naik Vaishali,Paulot FabienORCID,Stier PhilipORCID,Wild MartinORCID,Myhre GunnarORCID,Schulz MichaelORCID

Abstract

Abstract. Anthropogenic aerosols exert a cooling influence that offsets part of the greenhouse gas warming. Due to their short tropospheric lifetime of only several days, the aerosol forcing responds quickly to emissions. Here, we present and discuss the evolution of the aerosol forcing since 2000. There are multiple lines of evidence that allow us to robustly conclude that the anthropogenic aerosol effective radiative forcing (ERF) – both aerosol–radiation interactions (ERFari) and aerosol–cloud interactions (ERFaci) – has become less negative globally, i.e. the trend in aerosol effective radiative forcing changed sign from negative to positive. Bottom-up inventories show that anthropogenic primary aerosol and aerosol precursor emissions declined in most regions of the world; observations related to aerosol burden show declining trends, in particular of the fine-mode particles that make up most of the anthropogenic aerosols; satellite retrievals of cloud droplet numbers show trends in regions with aerosol declines that are consistent with these in sign, as do observations of top-of-atmosphere radiation. Climate model results, including a revised set that is constrained by observations of the ocean heat content evolution show a consistent sign and magnitude for a positive forcing relative to the year 2000 due to reduced aerosol effects. This reduction leads to an acceleration of the forcing of climate change, i.e. an increase in forcing by 0.1 to 0.3 W m−2, up to 12 % of the total climate forcing in 2019 compared to 1750 according to the Intergovernmental Panel on Climate Change (IPCC).

Funder

Horizon 2020

Deutsche Forschungsgemeinschaft

Publisher

Copernicus GmbH

Subject

Atmospheric Science

Reference154 articles.

1. Aas, W., Mortier, A., Bowersox, V., Cherian, R., Faluvegi, G., Fagerli, H., Hand, J., Klimont, Z., Galy-Lacaux, C., Lehmann, C. M. B., Lund Myhre, C., Myhre, G., Olivié, D., Sato, K., Quaas, J., Rao, P. S. P., Schulz, M., Shindell, D., Skeie, R. B., Stein, A., Takemura, T., Tsyro, S., Vet, R., and Xu, X.: Global and regional trends of atmospheric sulfur, Sci. Rep.-UK, 9, 953, https://doi.org/10.1038/s41598-018-37304-0, 2019. a, b, c, d, e, f, g

2. Albright, A. L., Proistosescu, C., and Huybers, P.: Origins of a Relatively Tight Lower Bound on Anthropogenic Aerosol Radiative Forcing from Bayesian Analysis of Historical Observations, J. Climate, 34, 8777–8792, https://doi.org/10.1175/JCLI-D-21-0167.1, 2021. a, b, c, d, e, f, g

3. Allen, M., Peters, G., Shine, K., Azar, C., Balcombe, P., Boucher, O., Cain, M., Ciais, P., Collins, W., Forster, P. M., Frame, D. J., Friedlingstein, P., Fyson, C., Gasser, T., Hare, B., Jenkins, S., Hamburg, S. P., Johansson, D. J. A., Lynch, J., Macey, A., Morfeldt, J., Nauels, A., Ocko, I., Oppenheimer, M., Pacala, S. W., Pierrehumbert, R., Rogelj, J., Schaeffer, M., Schleussner, C. F., Shindell, D., Skeie, R. B., Smith, S. M., and Tanaka, K.: Indicate separate contributions of long-lived and short-lived greenhouse gases in emission targets, npj Clim. Atmos. Sci., 5, 5, https://doi.org/10.1038/s41612-021-00226-2, 2022. a

4. Allison, L. C., Palmer, M. D., Allan, R. P., Hermanson, L., Liu, C., and Smith, D. M.: Observations of planetary heating since the 1980s from multiple independent datasets, Environ. Res. Comm., 2, 101001, https://doi.org/10.1088/2515-7620/abbb39, 2020. a

5. Andela, N., Morton, D. C., Giglio, L., Chen, Y., van der Werf, G. R., Kasibhatla, P. S., DeFries, R. S., Collatz, G. J., Hantson, S., Kloster, S., Bachelet, D., Forrest, M., Lasslop, G., Li, F., Mangeon, S., Melton, J. R., Yue, C., and Randerson, J. T.: A human-driven decline in global burned area, Science, 356, 1356–1362, https://doi.org/10.1126/science.aal4108, 2017. a

Cited by 29 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

同舟云学术

1.学者识别学者识别

2.学术分析学术分析

3.人才评估人才评估

"同舟云学术"是以全球学者为主线,采集、加工和组织学术论文而形成的新型学术文献查询和分析系统,可以对全球学者进行文献检索和人才价值评估。用户可以通过关注某些学科领域的顶尖人物而持续追踪该领域的学科进展和研究前沿。经过近期的数据扩容,当前同舟云学术共收录了国内外主流学术期刊6万余种,收集的期刊论文及会议论文总量共计约1.5亿篇,并以每天添加12000余篇中外论文的速度递增。我们也可以为用户提供个性化、定制化的学者数据。欢迎来电咨询!咨询电话:010-8811{复制后删除}0370

www.globalauthorid.com

TOP

Copyright © 2019-2024 北京同舟云网络信息技术有限公司
京公网安备11010802033243号  京ICP备18003416号-3