Anomalous Hall effect and Fermi surface reconstruction in topological antiferromagnet candidate GdAuPb

Author:

Liu Yonglai12,Xu Xitong1ORCID,Huang Yuqing3,He Miao12,Zhao Haitian12,Zeng Qingqi1,Zou Youming1ORCID,Xi Chuanying1,Jia Shuang345ORCID,Qu Zhe12ORCID

Affiliation:

1. Anhui Key Laboratory of Low-Energy Quantum Materials and Devices, CAS Key Laboratory of Photovoltaic and Energy Conservation Materials, High Magnetic Field Laboratory of Chinese Academy of Sciences (CHMFL), HFIPS, CAS 1 , Hefei 230031, China

2. Science Island Branch of Graduate School, University of Science and Technology of China 2 , Hefei 230026, China

3. International Center for Quantum Materials, School of Physics, Peking University 3 , Beijing 100871, China

4. Interdisciplinary Institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials, Peking University 4 , Beijing 100871, China

5. CAS Center for Excellence in Topological Quantum Computation, University of Chinese Academy of Sciences 5 , Beijing 100190, China

Abstract

The combination of topology and magnetism has demonstrated great potential in the search of emergent quantum matters. In this study, we report the synthesis, magnetic, and electrical properties of GdAuPb, a rare-earth-based half-Heusler topological antiferromagnet candidate. Magnetization and specific heat studies reveal highly frustrated antiferromagnetic ordering of Gd at TN = 11.5 K. Interestingly, this material possesses a large, unsaturated magnetoresistance up to 800% below TN and anomalous Hall conductivity as large as 750 Ω−1cm−1 in the antiferromagnetic state. Moreover, the electric transports including the SdH quantum oscillation patterns all exhibit a sudden change around 9 T, indicating a field-driven quantum transition related to the Fermi surface reconstruction. These results suggest that GdAuPb is close to a topological critical point, which can be easily tuned via external parameters. Our study demonstrates a strong interplay between band topology and magnetism in GdAuPb and offers clues for material designs for topological antiferromagnets.

Funder

National Key Research and Development Program of China

National Natural Science Foundation of China

Chinese Academy of Sciences

Anhui Provincial Natural Science Foundation

CAS Key Lab of Photovoltaic and Energy Conservation Materials Fund

Publisher

AIP Publishing

Subject

Physics and Astronomy (miscellaneous)

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