Key role of short-lived halogens on global atmospheric oxidation during historical periods

Author:

Bossolasco Adriana12ORCID,Fernandez Rafael P.34,Li Qinyi5,Mahajan Anoop S.6,Villamayor Julián1,Barrera Javier A.78,Heard Dwayne E.9ORCID,Cuevas Carlos A.1ORCID,Caram Cyril10,Szopa Sophie10,Saiz-Lopez Alfonso1ORCID

Affiliation:

1. Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Blas Cabrera, CSIC, Madrid, Spain

2. Physics Institute of Northwest Argentina, National Research Council (INFINOA-CONICET), National University of Tucumán (UNT), Tucumán, Argentina

3. Institute for Interdisciplinary Science, National Research Council (ICB-CONICET), Mendoza, Argentina

4. School of Natural Sciences (FCEN), National University of Cuyo (UNCuyo), Mendoza, Argentina

5. Environment Research Institute, Shandong University, Qingdao, China

6. Indian Institute of Tropical Meteorology, Ministry of Earth Sciences, Pune, India

7. Research Institute for Physical Chemistry of Córdoba, National Research Council (INFIQC-CONICET), Córdoba, Argentina

8. Department of Physical Chemistry, School of Chemical Sciences, National University of Córdoba (UNC), Córdoba, Argentina

9. School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK

10. Laboratoire des Sciences du Climat et de l'Environnement, LSCE/IPSL, CEA-CNRS-UVSQ, Université Paris-Saclay, Gif-sur-Yvette, France

Abstract

Short-lived halogens (SLH) play a crucial role in reducing atmospheric oxidation over time, this effect is more pronounced in the pre-industrial period, primarily due to enhanced halogen reactivity under low-NOx conditions.

Funder

H2020 European Research Council

Publisher

Royal Society of Chemistry (RSC)

Reference69 articles.

1. IPCC , Climate Change 2021: the Physical Science Basis. Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change , 2021

2. Climate and Tropospheric Oxidizing Capacity

3. D. J.Jacob , Introduction to Atmospheric Chemistry , Princeton University Press , 1999

4. B. J.Finlayson-Pitts and J. N.Pitts , Atmospheric Chemistry: Fundamentals and Experimental Techniques , John Wiley , New York , 1986

5. The nitrate radical: Physics, chemistry, and the atmosphere

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