Highly active ruthenium sites stabilized by modulating electron-feeding for sustainable acidic oxygen-evolution electrocatalysis

Author:

Wang Kexin1,Wang Yali2,Yang Bin13,Li Zhongjian13ORCID,Qin Xuetao4,Zhang Qinghua1ORCID,Lei Lecheng13,Qiu Ming2ORCID,Wu Gang5ORCID,Hou Yang13ORCID

Affiliation:

1. Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China

2. Institute of Nanoscience and Nanotechnology, College of Physical Science and Technology, Central China Normal University, Wuhan 430079, China

3. Institute of Zhejiang University-Quzhou, 78 Jiuhua Boulevard North, Quzhou 324000, China

4. Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, College of Engineering and BIC-ESAT, Perking University, Beijing 100871, China

5. Department of Chemical and Biological Engineering, University at Buffalo, the State University of New York, Buffalo, NY, 14260, USA

Abstract

An electron-feeding modulation strategy is developed to stabilize the highly active ruthenium site and strengthen the adsorption of the OH* intermediate toward sustainable acidic water electrolysis.

Funder

Natural Science Foundation of Zhejiang Province

National Natural Science Foundation of China

Central University Basic Research Fund of China

Zhejiang University

Chinese Academy of Sciences

University at Buffalo

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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