Reconstruction of LiF-rich interphases through an anti-freezing electrolyte for ultralow-temperature LiCoO2 batteries

Author:

Liu Jipeng123ORCID,Yuan Botao1,He Niandong1,Dong Liwei2,Chen Dongjiang1,Zhong Shijie1,Ji Yuanpeng2,Han Jiecai1,Yang Chunhui23ORCID,Liu Yuanpeng1,He Weidong145ORCID

Affiliation:

1. National Key Laboratory of Science and Technology on Advanced Composites in Special Environments, and Center for Composite Materials and Structures, Harbin Institute of Technology, Harbin, 150080, China

2. MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin, 150001, China

3. State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin, 150001, China

4. Chongqing Research Institute, Harbin Institute of Technology, Chongqing 401151, China

5. School of Mechanical Engineering, Chengdu University, Chengdu, 610106, China

Abstract

With iso-butyl formate (IF) as anti-freezing agent, a fluorine–sulfur electrolyte is designed to achieve low coordination number, high desolvation energy and stable LiF-rich interphase, and enables the stable operation of an electric fan at −70 °C.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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