Recent progress with one-dimensional metal halide perovskites: from rational synthesis to optoelectronic applications

Abstract

AbstractMetal halide perovskites can be readily synthesized, they exhibit tunable physical properties and excellent performance, and they are heavily studied optoelectronic materials. Compared to the typical three-dimensional perovskites, morphological-level one-dimensional (1D) nanostructures enable charge transport and photon propagation with low exciton binding energies and long charge-carrier diffusion lengths, while molecular-level 1D nanostructures exhibit good compositional and structural flexibilities, highly tunable bandgaps, strong quantum confinement effects, and excellent ambient stabilities. The 1D natures of these emerging halide perovskites enhance the performance of optoelectronic devices. Herein, we highlight recent progress realized in the syntheses and characterizations of both morphological- and molecular-level 1D halide perovskites with tunable structures, compositions, and properties, as well as their photovoltaic, light-emission, and photodetection applications. In addition, current challenges, future prospects, and promising research directions are discussed to provide guidance in advancing the field of 1D perovskites.