Climatology of Polar Stratospheric Clouds Derived from CALIPSO and SLIMCAT

Author:

Li Douwang1,Wang Zhe1,Li Shun1,Zhang Jiankai1ORCID,Feng Wuhu23ORCID

Affiliation:

1. School of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, China

2. National Centre for Atmospheric Science (NCAS), University of Leeds, Leeds LS2 9PH, UK

3. Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds LS2 9JT, UK

Abstract

Polar stratospheric clouds (PSCs) play a crucial role in ozone depletion in the polar stratosphere. In this study, the space-based PSCs record from CALISPO and an offline three-dimensional chemical transport model (SLIMCAT) are used to analyze the PSCs in the Arctic and the Antarctic for the period 2006−2021. Observations indicate that the seasonal evolution of the Antarctic PSC area is similar from year to year. In contrast, the Arctic PSCs show large differences in seasonal variations of coverage and duration in different years. The SLIMCAT simulations effectively capture the seasonal and interannual variations of PSCs. However, the simulated PSC areas are larger than CALIPSO observations, which can be attributed to the relatively high instrumental detection threshold of CALIPSO. SLIMCAT can capture the zonal asymmetry of PSCs in both the Antarctic and Arctic, and it can reproduce a more accurate spatial distribution of PSCs when the PSC coverage area is larger. In addition, accurate simulation of HNO3 is important for PSC simulation. Because the simulation of denitrification processes is poor in SLIMCAT, which uses the thermodynamic equilibrium PSC scheme, the PSCs modeled by SLIMCAT are located at higher altitudes compared to the observation in the Antarctic, where the denitrification processes are strong. In contrast, for ice PSCs of which HNO3 is not required in calculations and the Arctic where denitrification is weak, the simulated PSC at different altitudes closely matches the observations.

Funder

National Natural Science Foundation of China

Fundamental Research Funds for the Central Universities

Publisher

MDPI AG

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