Modern Ni and Pd–Ni Catalysts Supported on Sn–Al Binary Oxide for Oxy‐Steam Reforming of Methanol-Reference-Cited by-同舟云学术

Modern Ni and Pd–Ni Catalysts Supported on Sn–Al Binary Oxide for Oxy‐Steam Reforming of Methanol

Published:2018-06-27 Issue:9 Volume:6 Page:1687-1699
ISSN:2194-4288
Container-title:Energy Technology
language:en
Short-container-title:Energy Tech

Author:

Mierczynski Pawel¹,Mierczynska Agnieszka²,Ciesielski Radoslaw¹,Maniukiewicz Waldemar¹,Rogowski Jacek¹,Maniecki Tomasz P.¹,Dubkov Sergey³,Sysa Artem³,Gromov Dmitry³,Szynkowska Malgorzata I.¹,Vasilev Krasimir⁴

Affiliation:

1. Institute of General and Ecological Chemistry Lodz University of Technology Zeromskiego 116 90-924 Lodz Poland

2. The Australian Wine Research Institute Waite Precinct Hartley Grove cnr Paratoo Road Urrbrae (Adelaide) SA 5064 Australia

3. National Research University of Electronic Technology Shokin Square, Zelenograd Moscow 124498 Russia

4. School of Engineering University of South Australia Mawson Lakes SA 5095 Adelaide Australia

Abstract

AbstractMonometallic Ni and bimetallic Pd–Ni catalysts supported on mono‐SnO2 and SnO2–Al2O3 binary oxide are prepared using a wet impregnation and subsequent impregnation method. The catalysts are tested in oxy‐steam reforming of methanol (OSRM) and characterized. The activity measurements show that palladium‐promoted nickel catalysts supported on SnO2–Al2O3 exhibit high activity, selectivity towards hydrogen formation, and stability. The effect of Pd on reducibility, surface acidity, and morphology of the Ni supported catalyst, as well as its catalytic properties in OSRM, are discussed in detail.

Publisher

Wiley

Link

https://onlinelibrary.wiley.com/doi/pdf/10.1002/ente.201700840

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