High-entropy nanoparticles: Synthesis-structure-property relationships and data-driven discovery-Reference-Cited by-同舟云学术

High-entropy nanoparticles: Synthesis-structure-property relationships and data-driven discovery

Published:2022-04-08 Issue:6589 Volume:376 Page:
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Yao Yonggang¹^ORCID,Dong Qi¹^ORCID,Brozena Alexandra¹^ORCID,Luo Jian²^ORCID,Miao Jianwei³^ORCID,Chi Miaofang⁴^ORCID,Wang Chao⁵^ORCID,Kevrekidis Ioannis G.⁵^ORCID,Ren Zhiyong Jason⁶^ORCID,Greeley Jeffrey⁷^ORCID,Wang Guofeng⁸^ORCID,Anapolsky Abraham⁹,Hu Liangbing¹¹⁰^ORCID

Affiliation:

1. Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742, USA.

2. Department of NanoEngineering, Program of Materials Science and Engineering, University of California San Diego, La Jolla, CA 92093, USA.

3. Department of Physics and Astronomy and California NanoSystems Institute, University of California, Los Angeles, Los Angeles, CA 90095, USA.

4. Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37932, USA.

5. Department of Chemical and Biomolecular Engineering, Johns Hopkins University, Baltimore, MD 21218, USA.

6. Department of Civil and Environmental Engineering and Andlinger Center for Energy and the Environment, Princeton University, Princeton, NJ 08544, USA.

7. School of Chemical Engineering, Purdue University, West Lafayette, IN 47907, USA.

8. Department of Mechanical Engineering and Materials Science, University of Pittsburgh, Pittsburgh, PA 15261, USA.

9. Toyota Research Institute, Los Altos, CA 94022, USA.

10. Center for Materials Innovation, University of Maryland, College Park, MD 20742, USA.

Abstract

High-entropy nanoparticles have become a rapidly growing area of research in recent years. Because of their multielemental compositions and unique high-entropy mixing states (i.e., solid-solution) that can lead to tunable activity and enhanced stability, these nanoparticles have received notable attention for catalyst design and exploration. However, this strong potential is also accompanied by grand challenges originating from their vast compositional space and complex atomic structure, which hinder comprehensive exploration and fundamental understanding. Through a multidisciplinary view of synthesis, characterization, catalytic applications, high-throughput screening, and data-driven materials discovery, this review is dedicated to discussing the important progress of high-entropy nanoparticles and unveiling the critical needs for their future development for catalysis, energy, and sustainability applications.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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