Bottom-up construction of a superstructure in a porous uranium-organic crystal-Reference-Cited by-同舟云学术

Bottom-up construction of a superstructure in a porous uranium-organic crystal

Published:2017-05-12 Issue:6338 Volume:356 Page:624-627
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Li Peng¹^ORCID,Vermeulen Nicolaas A.¹,Malliakas Christos D.¹,Gómez-Gualdrón Diego A.²^ORCID,Howarth Ashlee J.¹^ORCID,Mehdi B. Layla³^ORCID,Dohnalkova Alice⁴^ORCID,Browning Nigel D.³⁵^ORCID,O’Keeffe Michael⁶,Farha Omar K.¹⁷^ORCID

Affiliation:

1. Department of Chemistry, Northwestern University, Evanston, IL 60208, USA.

2. Chemical and Biological Engineering Department, Colorado School of Mines, Golden, CO 80401, USA.

3. Physical and Computational Science Directorate, Pacific Northwest National Laboratory, Richland, WA 99352, USA.

4. Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, WA 99352, USA.

5. Materials Science and Engineering, University of Washington, Seattle, WA 98195, USA.

6. School of Molecular Sciences, Arizona State University, Tempe, AZ 85287, USA.

7. Department of Chemistry, Faculty of Science, King Abdulaziz University, Jeddah, Saudi Arabia.

Abstract

Intricacy anchored by uranium Metal-organic frameworks generally have one level of assembly complexity: Organic linkers join inorganic nodes in a repeating lattice. Li et al. created a structure composed of cuboctahedra, assembled from uranium cations and organic linkers, that shared triangular faces to form prisms. These structures formed cages, which in turn joined to make tetrahedra that assembled with a diamond-lattice topology. This hierarchical open structure generated a huge unit cell with more than 800 nodes and linkers, containing internal cavities with diameters of 5 and 6 nm. Science , this issue p. 624

Funder

National Science Foundation

U.S. Department of Energy

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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