High thermoelectric performance in low-cost SnS 0.91 Se 0.09 crystals

Author:

He Wenke1ORCID,Wang Dongyang1ORCID,Wu Haijun2ORCID,Xiao Yu1ORCID,Zhang Yang2ORCID,He Dongsheng3ORCID,Feng Yue3ORCID,Hao Yu-Jie3ORCID,Dong Jin-Feng4ORCID,Chetty Raju5ORCID,Hao Lijie6ORCID,Chen Dongfeng6ORCID,Qin Jianfei6ORCID,Yang Qiang7ORCID,Li Xin7ORCID,Song Jian-Ming7ORCID,Zhu Yingcai8ORCID,Xu Wei8ORCID,Niu Changlei9ORCID,Li Xin9,Wang Guangtao10ORCID,Liu Chang311ORCID,Ohta Michihiro5ORCID,Pennycook Stephen J.2ORCID,He Jiaqing3ORCID,Li Jing-Feng4ORCID,Zhao Li-Dong1ORCID

Affiliation:

1. School of Materials Science and Engineering, Beihang University, Beijing 100191, China.

2. Department of Materials Science and Engineering, National University of Singapore, Singapore 117575, Singapore.

3. Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China.

4. Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China.

5. Research Institute for Energy Conservation, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568, Japan.

6. Department of Nuclear Physics, Neutron Scattering Laboratory, China Institute of Atomic Energy, Beijing 102413, China.

7. Key Laboratory of Neutron Physics and Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900, China.

8. Beijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China.

9. Department of Isotope, China Institute of Atomic Energy, Beijing 102413, China.

10. College of Physics and Materials Science, Henan Normal University, Xinxiang 453007, China.

11. Shenzhen Key Laboratory of Quantum Science and Engineering, Shenzhen Institute for Quantum Science and Engineering, Shenzhen 518055, China.

Abstract

Lower-cost thermoelectrics Thermoelectric materials convert heat to electricity, making them attractive for heat harvesting or cooling applications. However, many high-performance thermoelectrics are made of expensive or toxic materials. He et al. found that a material composed of primarily tin and sulfur could be optimized to have relatively good thermoelectric properties. Introducing about 10% selenium to tin sulfide helped tune these properties by electronic band manipulation. This material is a step toward more earth-abundant, less toxic, and lower-cost thermoelectrics than the telluride-based materials currently in use. Science , this issue p. 1418

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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