Design and Preparation of Magnetism-Driven Intelligent Hydrogel Actuators
Author:
Chang Y.-J.12, Zhou Q.3, Hou W.-H.1, Liang Y.-H.1, Ren L.4, Sun D.-H.5, Ren L.-Q.1
Affiliation:
1. State Key Laboratory of Automotive Simulation and Control, Jilin University , Changchun , PRC 2. College of Food Science and Engineering, Jilin University , Changchun , PRC 3. Cadre’s Ward, The First Hospital of Jilin University , Changchun , PRC 4. School of Mechanical, Aerospace and Civil Engineering, University of Manchester , Manchester , UK 5. College of Science, Changchun Institute of Technology , Changchun , PRC
Abstract
Abstract
Novel kinds of magnetism-driven poly N,N-dimethylacrylamide bilayer intelligent hydrogels with various nanofibrillated cellulose (NFC) contents were prepared successfully via one-step insitu free radical polymerization. The bilayer hydrogels possessed high mechanical strength, efficient swelling and steady magnetic response. With the increase of nanofibrillated cellulose content, the crosslinking density of the hydrogels increased, leading to the decrease of swelling rate and increase of mechanical strength and swelling bending degree of hydrogel actuators, respectively. Fe3O4 particles existed tightly on the micropore surfaces of the hydrogels, which built the function base of magnetic response of hydrogel actuators. The addition of Fe3O4 was irrelevant to the variation of crosslinking density. The bilayer structure exhibited high bonding strength. Based on intelligent responsive properties, bilayer hydrogels were designed as soft magnetism-driven actuators, realizing capture and transportation properties and provided material candidates for soft robots.
Publisher
Walter de Gruyter GmbH
Subject
Materials Chemistry,Industrial and Manufacturing Engineering,Polymers and Plastics,General Chemical Engineering
Reference23 articles.
1. Bassik, N., Abebe, B. T., Laflin, K. E. and Gracias, D. H., “Photolitho-graphically Patterned Smart Hydrogel Based Bilayer Actuators", Polymer, 51, 6093 –6098 (2010), DOI:10.1016/j.polymer.2010.10.035 2. Feng, Y. Y., Qin, M. M., Guo, H. Q., Yoshino, K. and Feng, W., “Infrared-Actuated Recovery of Polyurethane Filled by Reduced Graphene Oxide/Carbon Nanotube Hybrids with High Energy Density", Acs Appl. Mater. Inter., 5, 10882–10888 (2013), DOI:10.1021/am403071k 3. Gao, Y., Wei, Z., Li, F., Yang, Z. M., Chen, Y. M., Zrinyi, M. and Osada, Y., “Synthesis of a Morphology Controllable Fe3O4 Nanoparticle/Hydrogel Magnetic Nanocomposite Inspired by Magnetotactic Bacteria and Its Application in H2O2 Detection", Green Chem., 16, 1255–1261 (2014), DOI:10.1039/C3GC41535J 4. Han, D., Farino, C., Yang, C., Scott, T., Browe, D., Choi, W., Freeman, J., W. and Lee, H., “Soft Robotic Manipulation and Locomotion with 3D Printed Electroactive Hydrogel", ACS Appl. Mater. Int., 10, 17512–17518 (2018), DOI:10.1021/acsami.°b04250 5. Haraguchi, K., Takehisa, T. and Fan, S., “Effects of Clay Content on the Properties of Nanocomposite Hydrogels Composed of Poly(Nisopropylacrylamide) and Clay", Macromolecules, 35, 10162 – 10171 (2002), DOI:10.1021/ma021301r
Cited by
1 articles.
订阅此论文施引文献
订阅此论文施引文献，注册后可以免费订阅5篇论文的施引文献，订阅后可以查看论文全部施引文献
|
|