Effects of nitrogen flow on the microstructure and mechanical properties of (TiZrNbMoTa)N high-entropy nitride films by magnetron sputtering

Author:

Liu Yuanpeng1ORCID,Nie Kaishan1ORCID,Tian Shuai12ORCID,Zhang Zhengyi1ORCID,Li Zheng1ORCID,Wang Dong1ORCID,Hu Jibo1ORCID

Affiliation:

1. School of Mechanical Engineering, Zhengzhou University of Aeronautics 1 , Zhengzhou 450046, People’s Republic of China

2. Henan Key Laboratory of General Aviation Technology, Zhengzhou University of Aeronautics 2 , Zhengzhou 450046, People’s Republic of China

Abstract

The binary nitride coatings corresponding to Ti, Zr, Nb, Mo, and Ta have good thermal stability, hardening wear resistance, and high-temperature oxidation resistance. Therefore, the high-entropy alloy nitride coating composed of these five elements is expected to show excellent mechanical properties, and it is suitable for extending tool life in dry-cutting environments. In this paper, (TiZrNbMoTa)Nx high-entropy nitride films were synthesized using a multitarget nonequilibrium magnetron sputtering technique. The paper aimed at investigating the effects of different nitrogen flow rates (FN) on the microstructure and mechanical properties of the films. The results show that, with the increase in FN, the deposition rate gradually decreased, the films exhibited a face-centered cubic structure, and the grain gradually changed from coarse columnar crystals to ultrafine grain structures. The hardness, elastic modulus, and binding force all showed a tendency to increase and then decreased with increasing FN. The hardness and elastic modulus reached their maximum values of 34.39 and 400.97 GPa, respectively, at an FN of 60 SCCM, and the formation of covalent bonds and grain refinement promoted the increase in hardness. This research provided a theoretical foundation for designing and preparing high-entropy ceramic coatings with high performance.

Funder

Henan Provincial Science and Technology Research Project

Henan Province University Innovation Talents Support Program

National College Students Innovation and Entrepreneurship Training Program

Open fund of Henan Key Laboratory of General Aviation Technology

Zhengzhou University of Aeronautics Graduate Education Innovation Program Fund Project

Publisher

American Vacuum Society

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